Zarif who arrived in Yerevan on Wednesday morning met and held talks with his Armenian counterpart Ara Ayvazyan.
He is scheduled to meet with Acting Prime Minister Nikol Pashinyan and Armenian President Armen Sargsyan.
Iranian foreign minister met with the President of Azerbaijan Republic Ilham Aliyev in Baku on Tuesday.
Expressing satisfaction with the expanding trend and the appropriate level of relations between the two countries in recent years, the two sides emphasized the development and deepening of relations between Tehran and Baku.
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