Zarif is scheduled to meet with EU Foreign Policy Chief Federica Mogherini as well as French FM Laurent Fabius, British Foreign Secretary Philip Hammond and German FM Frank-Walter Steinmeier.
They will hold talks on drafting a final comprehensive agreement over Iran's nuclear program.
Iranian Deputy FMs Seyed Abbas Araghchi and Majid Takht-Ravanchi who are currently in Vienna, will join Zarif in Luxembourg.
Over the past month, Iran's Zarif has held talks with US Secretary of State John Kerry in Geneva as well as Russian and Chinese FMs in Moscow.
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